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Journal Articles

Hydrogen analyses of titanium hydride by ERD and NRG methods

Tsuchiya, Bun*; Teshigawara, Makoto; Nagata, Shinji*; Konashi, Kenji*; Yasuda, Ryo; Nishino, Yasuharu; Nakagawa, Tetsuya*; Yamawaki, Michio*

Nuclear Instruments and Methods in Physics Research B, 190(1-4), p.699 - 703, 2002/05

 Times Cited Count:10 Percentile:54.86(Instruments & Instrumentation)

Practicability of Elastic Recoil Detection (ERD) and Neutron Radiography (NRG) methods for hydrogen concentration in titanium hydrides (d-TiHx : 1.6<x<2.0) is investigated. In ERD methods, the hydrogen concentration in the surface of TiHx is recognized. In NRG method, the hydrogen concentration over the balk was confirmed. These results show that both methods are effective means for estimating the hydrogen concentration in hydride materials.

JAEA Reports

Determination of neptunium in neptunium-uranium-plutonium mixed oxide fuel by spectrophotometry.

; ; ; ; ; *; *

JNC TN8400 2001-026, 29 Pages, 2001/12

JNC-TN8400-2001-026.pdf:0.99MB

The measurement condition by spectrophotometry was evaluated to measure Np content in MOX fuel containing Np. The Np concentration was obtained by measuring the 727nm absorption peak, after the valence of Np in the sample solution was adjusted to the Np(Ⅳ). The calibration curve showed the linearity up to Np concentration 0.8mg/ml. Though Pu and U quantity were respectively added to the Np solution to 30 times and 60 times of Np concentration, there was no effect to the Np analysis. By using this method, relative standard deviation (RSD) of the analyzed values of Np content for 2%Np - MOX fuel was about 4%. In addition, It was confirmed that the Np content could be measured without separating Np from Pu and U. This method can be sufficiently applied as a quick simple method to analyze Np content in MOX fuel containing Np.

JAEA Reports

Evaluation of the analytical errors jn plutonium and uranium isotopic composition analysis based on routine control measurement data (1998/9$$sim$$2000/12)

Kobayashi, Hideo; ; ; ; ; *; *

JNC TN8440 2001-005, 33 Pages, 2001/02

JNC-TN8440-2001-005.pdf:1.24MB

Four mass spectrometers are used for plutonium and uranium isotopic composition analysis in the Plutonium Fuel Center. Analytical errors of the analysis was evaluated based on routine control data obtained with measurement of reference materials. It was confirmed that the errors satisfied the International Target Values for safeguard analysis, and the random error of the analysis was improved by changing conventional method to total evaporation method.

JAEA Reports

Improvement of the technique for stack monitoring based on behavior analysis of natural radio-nuclides; The technique for reducing the value of the exhaust monitor's background

Izaki, Kenji; Noda, Kimio; ; Kashimuta, Yoshio*

JNC TN8410 2001-005, 30 Pages, 2001/01

JNC-TN8410-2001-005.pdf:0.62MB

Stack monitoring is the most important work in radiation control works. Exhaust monitors used for stack monitoring have the background (which is the counts by natural radio-nuclides) on normal condition, and the values of the background vary with the facilities. Therefore, if the value of background is high, it is difficult to estimate rapidly the radioactive concentration in the exhaust. In order to estimate rapidly the radioactive concentration in exhaust, we analyzed the behavior of natural radioactivity in the facilities and examine the technique fo reducing the value of the background. As a result of the examination, we found that it is possible to estimate rapidly if we change over the monitoring point to immediately after the HEPA filters on the exhaust duct. In this reports, the analyzed results of behavior of natural radio-nuclides in the facilities and the technique for reducing the values of the background are described. To reduce the value of the background has a major effect on not only rapidly estimating the radioactive density in the exhaust but also finding the unusual things on stack monitoring.

JAEA Reports

Organic acid dissolving in groundwater in the Mobara gas field

JNC TN8400 2000-030, 17 Pages, 2000/12

JNC-TN8400-2000-030.pdf:0.44MB

As a representative of natural marine groundwater, the author selected pumped water from a Quaternary sedimentary aquifer of the Mobara gas-field in Japan and measured the concentration of total organic carbon (TOC) and of organic acid anions (formic, acetic, lactic, succinic, humic, fulvic, propionic, valeric and butyric acids). The concentration of TOC ranged from 22$$pm$$1 to 24$$pm$$0mg/L. As organic acid anions, only succinic and fulvic acids were detected and each concentration was given to be from 5.8$$pm$$ 0.5 to 8.3$$pm$$0.3 and from 3.3$$pm$$0.2 to 3.5$$pm$$0.2mg/L, respectively. By consideration of the temperature and the [SO$$_{4}$$$$^{2-}$$] of the groundwater, it is inferred that the organic acid has been significantly decomposed by activities of microbes, such as the fermentation process, CH$$_{3}$$COO$$^{-}$$ + H$$_{2}$$O = HCO$$_{3}$$$$^{-}$$ + CH$$_{4}$$.

JAEA Reports

Detailed investigation on the environmental effects from the liquid effluent of JNC reprocessing plant (IV); (April, 1996$$sim$$March, 2000)

; Shinohara, Kunihiko; ; ; ; Isozaki, Tokuju; ; *

JNC TN8440 2000-003, 93 Pages, 2000/08

JNC-TN8440-2000-003.pdf:2.2MB

The investigation on the radioactivity concentration for gross beta, $$^{3}$$H and $$^{137}$$Cs in seawater collected around the discharge point had been performed in order to grasp the change of the activity level of the coastal seawater offshore the JNC Tokai Works from the low level liquid effluent of the reprocessing plant. After the investigation on the radioactivity in seawater during the hot examination, the detailed investigation on the environmental effects from the liquid effluent of JNC reprocessing plant has been performed since July 1978 on the basis of the request from Ibaraki prefecture as the full-scale operation of the reprocessing plant. Consequently, no increase of the radioactive concentration due to the discharged effluent has been observed. And also, as the result of the consideration to the investigation on the environmental effect from the liquid effluent throughout 22 years since 1978, no change of the radioactive concentration level in seawater was recognized.

JAEA Reports

Measurement of U and Pu concentration by X-ray fluorescence spectrometry using vertical irradiation system.

; ; ; Ikeda, Hisashi ; Jitsukata, Shu*; *

JNC TN8410 2000-022, 55 Pages, 2000/05

JNC-TN8410-2000-022.pdf:1.57MB

Measurement of U and Pu concentrations by wavelength dispersion type X-ray fluorescence spectrometry was studied. Sample holder was installed inside of glove box and other instruments, X-ray tube, monochromator and detectors were set out side of the glove box. X-rays was irradiated to sample though Be window. Fluorescent X-rays form sample were also passing though the same Be window and detected outside. Analytical conditions were optimized as follows. Sample thickness is 8 mm, which is 3ml of sample volume by the sample holder. Voltage and eurrent for X-ray tube is 50kV and 40 mA, respectively. Measurement was done twice, 60 seconds each, and averaged X-ray intensity was used to calculate elemental concentrations. Matrix correction was necessary to measure U and Pu concentration within 10% accuracy. Detection limits were calculated to 0.4 mg/L for U and 0.7mg/L for Pu. Calibration curve was liner up to 9 g/L fbr U and Pu. Two calculation methods, calibration curve method and standard addition method, were studied to measure Pu concentration in organic solution. Detection limit was 5.3 mg/L and 0.2 mg/L, respectively.

JAEA Reports

JOYO coolant sodium and cover gas purity control database (MK-II core)

; ; Saikawa, Takuya*; Sukegawa, Kazuya*

JNC TN9410 2000-008, 66 Pages, 2000/03

JNC-TN9410-2000-008.pdf:1.39MB

The experimental fast reactor "JOYO" served as the MK-II irradiation bed core for testing fuel and material for FBR development for 15 years from 1982 to 1997. During the MK-II operation, impurities concentrations in the sodium and the argon gas were determined by 67 samples of primary sodium, 81 samples of secondary sodium, 75 samples of primary argon gas, 89 samples of secondary argon gas (the overflow tank) and 89 samples of secondary argon gas (the dump tank). The sodium and the argon gas purity control data were accumulated from in thirty-one duty operations, thirteen special test operations and eight annual inspections. These purity control results and related plant data were compiled into database, which were recorded on CD-ROM for user convenience. Purity control data include concentration of oxygen, carbon, hydrogen, nitrogen, chlorine, iron, nickel and chromium in sodium, concentration of oxygen, hydrogen, nitrogen, carbon monoxide, carbon dioxide, methane and helium in argon gas with the reactor condition.

JAEA Reports

None

*

JNC TJ7420 2000-001, 14 Pages, 2000/02

JNC-TJ7420-2000-001.pdf:0.27MB

no abstracts in English

JAEA Reports

None

Iida, Takao*

JNC TJ6400 2000-008, 58 Pages, 1999/03

JNC-TJ6400-2000-008.pdf:1.9MB

None

JAEA Reports

None

*; *

JNC TJ1400 99-030, 102 Pages, 1999/03

JNC-TJ1400-99-030.pdf:4.0MB

no abstracts in English

JAEA Reports

None

Kato, Toshihiro*; ; ; ; Ishibashi, Yuzo; Takeda, Seiichiro

PNC TN8410 98-070, 31 Pages, 1998/02

PNC-TN8410-98-070.pdf:0.99MB

None

JAEA Reports

None

PNC TJ1615 98-001, 58 Pages, 1998/02

PNC-TJ1615-98-001.pdf:1.98MB

no abstracts in English

JAEA Reports

Installation of aerosol behavior model into multi-dimensional thermaI hydraulic analysis code AQUA

; Yamaguchi, Akira

PNC TN9410 98-028, 33 Pages, 1997/12

PNC-TN9410-98-028.pdf:0.93MB

The safety analysis of FBR plant system for sodium leak phenomena needs to evaluate the deposition of the aerosol particle to the components in the plant, the chemical reaction of aerosol to humidity in the air and the effect of the combustion heat through aerosol to the structural component. For this purpose, ABC-INTG (Aerosol Behavior in Containment-INTeGrated Version) code has been developed and used until now. This code calculates aerosol behavior in the gas area of uniform temperature and pressure by 1 cell-model. Later, however, more detailed calculation of aerosol behavior requires the installation of aerosol model into multi-cell thermal hydraulic analysis code AQUA. AQUA can calculate the carrier gas flow, temperature and the distribution of the aerosol spatial concentration. On the other hand, ABC-INTG can calculate the generation, deposition to the wall and flower, agglomeration of aerosol particle and figure out the distribution of the aerosol particle size. Thus, the combination of these two codes enables to deal with aerosol model coupling the distribution of the aerosol spatial concentration and that of the aerosol particle size. AQUA and ABC-INTG were developed separately, therefore, several subroutine were modified and composed. Especially, the interface program which exchanges data between these two codes is important to execute transient calculation. This report describes aerosol behavior model, how to install the aerosol model to AQUA and new subroutine equipped to the code. Furthermore, the test calculations of the simple structural model were executed by this code, appropriate results were obtained. Thus, this code has prospect to predict aerosol behavior by the introduction of coupling analysis with multi-dimensional gas thermo-dynamics for sodium combustion evaluation.

JAEA Reports

None

PNC TN1410 97-041, 29 Pages, 1997/11

PNC-TN1410-97-041.pdf:1.35MB

no abstracts in English

JAEA Reports

None

PNC TJ1615 97-001, 5 Pages, 1997/03

PNC-TJ1615-97-001.pdf:0.32MB

no abstracts in English

JAEA Reports

None

PNC TJ1603 97-003, 80 Pages, 1997/03

PNC-TJ1603-97-003.pdf:3.22MB

no abstracts in English

JAEA Reports

None

PNC TN1410 96-057, 56 Pages, 1996/10

PNC-TN1410-96-057.pdf:1.66MB

no abstracts in English

JAEA Reports

None

*; *; *

PNC TJ1645 96-001, 57 Pages, 1996/02

PNC-TJ1645-96-001.pdf:2.0MB

no abstracts in English

31 (Records 1-20 displayed on this page)